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On December 14, 1837, the second Congress of the Republic of Texas adjusted geographical limits to create Fayette County, and remove Gonzales and Caldwell Counties from Mina's boundaries. On December 18, 1837, Sam Houston signed acts that (a) incorporated the town of Mina and (b) changed the name of the county and town of Mina to Bastrop to honor Felipe Enrique Neri, Baron of Bastrop, an early Dutch settler who helped Stephen F. Austin obtain land grants in Texas.
On May 24, 1838, the Republic of Texas added parts of Kimble and Comal Counties to contain parts of present-day Blanco, Burnet, Williamson, Travis, Hays, Comal, Caldwell, Bastrop, Lee, Gonzales, and Fayette counties.
From January 25, 1840, to January 25, 1850, Bastrop county limits shifted nearly to its present dimensions, including small portions of Lee, Williamson, Caldwell, Gonzales and Fayette Counties.
In December 1942, Bastrop was the site of an alleged military murder, in which Sgt. Walter Springs was gunned down by a White military police officer following a dispute. Springs was shot in the back, but the case remains largely unsolved to this day. A memorial scholarship in his honor has been active at his alma mater, Regis University, for most of the period since 1952 and has the backing of former NBA All Star Chauncey Billups.
In September 2011, Bastrop County suffered the most destructive wildfire in Texas history, which destroyed over 1,600 homes.
In March 2022, the Refuge Ranch, a facility in rural Bastrop County for girls who had been victims of sexual trafficking, was ordered closed down after allegations that the girls had been subjected to further exploitation by ranch staffers.